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A regional air quality forecasting system over Europe: the MACC-II daily ensemble production

机译:欧洲区域空气质量预报系统:maCC-II日常集合生产

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摘要

This paper describes the pre-operational analysis and forecasting system developed during MACC (Monitoring Atmospheric Composition and Climate) and continued in the MACC-II (Monitoring Atmospheric Composition and Climate: Interim Implementation) European projects to provide air quality services for the European continent. This system is based on seven state-of-the art models developed and run in Europe (CHIMERE, EMEP, EURAD-IM, LOTOS-EUROS, MATCH, MOCAGE and SILAM). These models are used to calculate multi-model ensemble products. The paper gives an overall picture of its status at the end of MACCII (summer 2014) and analyses the performance of the multi-model ensemble. The MACC-II system provides daily 96 h forecasts with hourly outputs of 10 chemical species/aerosols (O-3, NO2, SO2, CO, PM10, PM2.5, NO, NH3, total NMVOCs (non-methane volatile organic compounds) and PAN + PAN precursors) over eight vertical levels from the surface to 5 km height. The hourly analysis at the surface is done a posteriori for the past day using a selection of representative air quality data from European monitoring stations. The performance of the system is assessed daily, weekly and every 3 months (seasonally) through statistical indicators calculated using the available representative air quality data from European monitoring stations. Results for a case study show the ability of the ensemble median to forecast regional ozone pollution events. The seasonal performances of the individual models and of the multi-model ensemble have been monitored since September 2009 for ozone, NO2 and PM10. The statistical indicators for ozone in summer 2014 show that the ensemble median gives on average the best performances compared to the seven models. There is very little degradation of the scores with the forecast day but there is a marked diurnal cycle, similarly to the individual models, that can be related partly to the prescribed diurnal variations of anthropogenic emissions in the models. During summer 2014, the diurnal ozone maximum is underestimated by the ensemble median by about 4 mu g m(-3) on average. Locally, during the studied ozone episodes, the maxima from the ensemble median are often lower than observations by 30-50 mu g m(-3). Overall, ozone scores are generally good with average values for the normalised indicators of 0.14 for the modified normalised mean bias and of 0.30 for the fractional gross error. Tests have also shown that the ensemble median is robust to reduction of ensemble size by one, that is, if predictions are unavailable from one model. Scores are also discussed for PM10 for winter 2013-1014. There is an underestimation of most models leading the ensemble median to a mean bias of 4.5 mu g m(-3). The ensemble median fractional gross error is larger for PM10 (similar to 0.52) than for ozone and the correlation is lower (similar to 0.35 for PM10 and similar to 0.54 for ozone). This is related to a larger spread of the seven model scores for PM10 than for ozone linked to different levels of complexity of aerosol representation in the individual models. In parallel, a scientific analysis of the results of the seven models and of the ensemble is also done over the Mediterranean area because of the specificity of its meteorology and emissions. The system is robust in terms of the production availability. Major efforts have been done in MACC-II towards the operationalisation of all its components. Foreseen developments and research for improving its performances are discussed in the conclusion.
机译:本文介绍了在MACC(监测大气成分和气候)期间开发并在MACC-II(监测大气成分和气候:临时实施)欧洲项目中开发的运行前分析和预测系统,该项目旨在为欧洲大陆提供空气质量服务。该系统基于在欧洲开发和运行的七个最新模型(CHIMERE,EMEP,EURAD-IM,LOTOS-EUROS,MATCH,MOCAGE和SILAM)。这些模型用于计算多模型集成产品。本文概述了其在MACCII结束时(2014年夏季)的状况,并分析了多模型集成的性能。 MACC-II系统每天提供96小时预报,每小时输出10种化学物质/气溶胶(O-3,NO2,SO2,CO,PM10,PM2.5,NO,NH3,总NMVOC(非甲烷挥发性有机化合物)和PAN + PAN前体)从地表到5 km高的八个垂直高度上。在过去的一天中,使用欧洲监测站提供的代表性空气质量数据进行选择,在过去的一天中对地面每小时进行一次分析。该系统的性能每天,每周和每3个月(季节性)通过统计指标进行评估,这些指标使用欧洲监测站提供的代表性空气质量数据计算得出。案例研究的结果表明,集合中位数能够预测区域性臭氧污染事件。自2009年9月以来,已经监测了各个模型和多模型集合的季节性性能,包括臭氧,NO2和PM10。 2014年夏季的臭氧统计指标显示,与七个模型相比,集合中位数平均表现出最佳性能。与预报日相比,分数几乎没有降级,但是与各个模型相似,其昼夜周期明显,这部分与模型中人为排放的规定昼夜变化有关。在2014年夏季,集合臭氧层的中位数低估了每日最大臭氧浓度,平均降低了约4μg m(-3)。在当地,在研究的臭氧事件中,集合中值的最大值通常比观测值低30-50μg m(-3)。总体而言,臭氧分数通常较好,归一化指标的平均值为0.14,修正的平均偏差为0.30,小数总误差为0.30。测试还显示,合奏中位数对于将合奏大小减小1(即,如果无法从一种模型获得预测)具有鲁棒性。还讨论了2013-1014年冬季PM10的得分。大多数模型都低估了整体中位数,导致平均偏差为4.5μg m(-3)。 PM10的总体中位数总误差大于臭氧(近似于0.52),相关性较低(PM10近似于0.35,臭氧近似于0.54)。这与PM10的七个模型得分的散布比臭氧的更大散布有关,后者与各个模型中气溶胶表示的不同复杂程度有关。同时,由于其气象学和排放的特殊性,还对地中海地区的七个模型和整体结果进行了科学分析。该系统在生产可用性方面很强大。 MACC-II在其所有组件的操作方面已经做出了重大努力。结论中讨论了可预见的发展和改进其性能的研究。

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